A numerical study on gas-liquid mass transfer in the rotor-stator spinning disc reactor

K.M.P. van Eeten; R. Verzicco; J. van der Schaaf; G.J.F. van Heijst; J.C. Schouten

doi:10.1016/j.ces.2015.02.020

A numerical study on gas-liquid mass transfer in the rotor-stator spinning disc reactor

K.M.P. van Eeten
, R. Verzicco
, J. van der Schaaf
, G.J.F. van Heijst
, J.C. Schouten^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › Academic › peer-review

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Abstract

The gas-liquid mass transfer coefficient was investigated in a novel multiphase reactor: the rotor-stator spinning disc reactor. Direct Numerical Simulations of the flow field around a single bubble in the reactor showed that vortex stretching invoked the presence of turbulence inside the thin liquid film surrounding the bubble. The Direct Numerical Simulations further provided a measure for the eddy diffusivity in the thin liquid film caused by this increase in vorticity. An expression was subsequently derived from a mass balance using these eddy diffusivities in order to estimate the order of magnitude of gas-liquid mass transfer coefficients. These estimates were found to lie more in line with experimental results in literature than previously used mass transfer models based on Higbie's penetration theory.

Original language	English
Pages (from-to)	14-24
Number of pages	11
Journal	Chemical engineering science
Volume	129
DOIs	https://doi.org/10.1016/j.ces.2015.02.020
Publication status	Published - 6 Jun 2015

Keywords

Direct numerical simulation
Gas-liquid mass transfer
Hydrodynamics
Rotor-stator spinning disc reactor
2023 OA procedure

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10.1016/j.ces.2015.02.020

ArticleFinal published version, 2.11 MBLicence: Taverne

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title = "A numerical study on gas-liquid mass transfer in the rotor-stator spinning disc reactor",

abstract = "The gas-liquid mass transfer coefficient was investigated in a novel multiphase reactor: the rotor-stator spinning disc reactor. Direct Numerical Simulations of the flow field around a single bubble in the reactor showed that vortex stretching invoked the presence of turbulence inside the thin liquid film surrounding the bubble. The Direct Numerical Simulations further provided a measure for the eddy diffusivity in the thin liquid film caused by this increase in vorticity. An expression was subsequently derived from a mass balance using these eddy diffusivities in order to estimate the order of magnitude of gas-liquid mass transfer coefficients. These estimates were found to lie more in line with experimental results in literature than previously used mass transfer models based on Higbie's penetration theory.",

keywords = "Direct numerical simulation, Gas-liquid mass transfer, Hydrodynamics, Rotor-stator spinning disc reactor, 2023 OA procedure",

author = "\{van Eeten\}, K.M.P. and R. Verzicco and \{van der Schaaf\}, J. and \{van Heijst\}, G.J.F. and J.C. Schouten",

note = "Funding Information: The authors gratefully acknowledge the European Research Council (ERC) for their financial support to this project (ERC Contract 227010 ). Publisher Copyright: {\textcopyright} 2015 Elsevier Ltd.",

year = "2015",

month = jun,

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doi = "10.1016/j.ces.2015.02.020",

language = "English",

volume = "129",

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AU - van Eeten, K.M.P.

AU - Verzicco, R.

AU - van der Schaaf, J.

AU - van Heijst, G.J.F.

AU - Schouten, J.C.

N1 - Funding Information: The authors gratefully acknowledge the European Research Council (ERC) for their financial support to this project (ERC Contract 227010 ). Publisher Copyright: © 2015 Elsevier Ltd.

PY - 2015/6/6

Y1 - 2015/6/6

N2 - The gas-liquid mass transfer coefficient was investigated in a novel multiphase reactor: the rotor-stator spinning disc reactor. Direct Numerical Simulations of the flow field around a single bubble in the reactor showed that vortex stretching invoked the presence of turbulence inside the thin liquid film surrounding the bubble. The Direct Numerical Simulations further provided a measure for the eddy diffusivity in the thin liquid film caused by this increase in vorticity. An expression was subsequently derived from a mass balance using these eddy diffusivities in order to estimate the order of magnitude of gas-liquid mass transfer coefficients. These estimates were found to lie more in line with experimental results in literature than previously used mass transfer models based on Higbie's penetration theory.

AB - The gas-liquid mass transfer coefficient was investigated in a novel multiphase reactor: the rotor-stator spinning disc reactor. Direct Numerical Simulations of the flow field around a single bubble in the reactor showed that vortex stretching invoked the presence of turbulence inside the thin liquid film surrounding the bubble. The Direct Numerical Simulations further provided a measure for the eddy diffusivity in the thin liquid film caused by this increase in vorticity. An expression was subsequently derived from a mass balance using these eddy diffusivities in order to estimate the order of magnitude of gas-liquid mass transfer coefficients. These estimates were found to lie more in line with experimental results in literature than previously used mass transfer models based on Higbie's penetration theory.

KW - Direct numerical simulation

KW - Gas-liquid mass transfer

KW - Hydrodynamics

KW - Rotor-stator spinning disc reactor

KW - 2023 OA procedure

UR - https://www.scopus.com/pages/publications/84924126872

U2 - 10.1016/j.ces.2015.02.020

DO - 10.1016/j.ces.2015.02.020

M3 - Article

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VL - 129

SP - 14

EP - 24

JO - Chemical engineering science

JF - Chemical engineering science

ER -

A numerical study on gas-liquid mass transfer in the rotor-stator spinning disc reactor

Abstract

Keywords

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