Background-free nonlinear microspectroscopy with vibrational molecular interferometry

E.T. Garbacik; Jeroen P. Korterik; Cornelis Otto; S. Mukamel; Jennifer Lynn Herek; Herman L. Offerhaus

doi:10.1117/12.908158

Background-free nonlinear microspectroscopy with vibrational molecular interferometry

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

1 Citation (Scopus)

11 Downloads (Pure)

Abstract

We demonstrate a method for performing nonlinear microspectroscopy that provides an intuitive and unified description of the various signal contributions, and allows the direct extraction of the vibrational response. Three optical fields create a pair of Stokes Raman pathways that interfere in the same vibrational state. Frequency modulating one of the fields leads to amplitude modulations on all of the fields. This vibrational molecular interferometry (VMI) technique allows imaging at high speed free of non-resonant background, and is able to distinguish between electronic and vibrational contributions to the total signal

Original language	English
Title of host publication	Multiphoton Microscopy in the Biomedical Sciences XII
Subtitle of host publication	22–24 January 2012, San Francisco, California, United States
Editors	Ammasi Periasamy, Karsten König, Peter T.C. So
Publisher	SPIE
ISBN (Print)	9780819488695
DOIs	https://doi.org/10.1117/12.908158
Publication status	Published - 9 Feb 2012
Event	SPIE BiOS 2012 - The Moscone Center, San Francisco, United States Duration: 21 Jan 2012 → 26 Jan 2012

Publication series

Name	Proceedings of SPIE
Publisher	SPIE
Volume	8226
ISSN (Print)	0277-786X

Conference

Conference	SPIE BiOS 2012
Country/Territory	United States
City	San Francisco
Period	21/01/12 → 26/01/12

Keywords

METIS-286037
IR-84664

Access to Document

10.1117/12.908158

Cite this

Garbacik, E. T., Korterik, J. P., Otto, C., Mukamel, S., Herek, J. L., & Offerhaus, H. L. (2012). Background-free nonlinear microspectroscopy with vibrational molecular interferometry. In A. Periasamy, K. König, & P. T. C. So (Eds.), Multiphoton Microscopy in the Biomedical Sciences XII: 22–24 January 2012, San Francisco, California, United States Article 822605 (Proceedings of SPIE; Vol. 8226). SPIE. https://doi.org/10.1117/12.908158

@inproceedings{83b640bec9964a7e80c765b176e2585e,

title = "Background-free nonlinear microspectroscopy with vibrational molecular interferometry",

abstract = "We demonstrate a method for performing nonlinear microspectroscopy that provides an intuitive and unified description of the various signal contributions, and allows the direct extraction of the vibrational response. Three optical fields create a pair of Stokes Raman pathways that interfere in the same vibrational state. Frequency modulating one of the fields leads to amplitude modulations on all of the fields. This vibrational molecular interferometry (VMI) technique allows imaging at high speed free of non-resonant background, and is able to distinguish between electronic and vibrational contributions to the total signal",

keywords = "METIS-286037, IR-84664",

author = "E.T. Garbacik and Korterik, \{Jeroen P.\} and Cornelis Otto and S. Mukamel and Herek, \{Jennifer Lynn\} and Offerhaus, \{Herman L.\}",

year = "2012",

month = feb,

day = "9",

doi = "10.1117/12.908158",

language = "English",

isbn = "9780819488695",

series = "Proceedings of SPIE",

publisher = "SPIE",

editor = "Ammasi Periasamy and Karsten K{\"o}nig and So, \{Peter T.C.\}",

booktitle = "Multiphoton Microscopy in the Biomedical Sciences XII",

address = "United States",

note = "SPIE BiOS 2012 ; Conference date: 21-01-2012 Through 26-01-2012",

}

Garbacik, ET, Korterik, JP , Otto, C, Mukamel, S, Herek, JL & Offerhaus, HL 2012, Background-free nonlinear microspectroscopy with vibrational molecular interferometry. in A Periasamy, K König & PTC So (eds), Multiphoton Microscopy in the Biomedical Sciences XII: 22–24 January 2012, San Francisco, California, United States., 822605, Proceedings of SPIE, vol. 8226, SPIE, SPIE BiOS 2012, San Francisco, California, United States, 21/01/12. https://doi.org/10.1117/12.908158

Background-free nonlinear microspectroscopy with vibrational molecular interferometry. / Garbacik, E.T.; Korterik, Jeroen P.; Otto, Cornelis et al.
Multiphoton Microscopy in the Biomedical Sciences XII: 22–24 January 2012, San Francisco, California, United States. ed. / Ammasi Periasamy; Karsten König; Peter T.C. So. SPIE, 2012. 822605 (Proceedings of SPIE; Vol. 8226).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

TY - GEN

T1 - Background-free nonlinear microspectroscopy with vibrational molecular interferometry

AU - Garbacik, E.T.

AU - Korterik, Jeroen P.

AU - Otto, Cornelis

AU - Mukamel, S.

AU - Herek, Jennifer Lynn

AU - Offerhaus, Herman L.

PY - 2012/2/9

Y1 - 2012/2/9

N2 - We demonstrate a method for performing nonlinear microspectroscopy that provides an intuitive and unified description of the various signal contributions, and allows the direct extraction of the vibrational response. Three optical fields create a pair of Stokes Raman pathways that interfere in the same vibrational state. Frequency modulating one of the fields leads to amplitude modulations on all of the fields. This vibrational molecular interferometry (VMI) technique allows imaging at high speed free of non-resonant background, and is able to distinguish between electronic and vibrational contributions to the total signal

AB - We demonstrate a method for performing nonlinear microspectroscopy that provides an intuitive and unified description of the various signal contributions, and allows the direct extraction of the vibrational response. Three optical fields create a pair of Stokes Raman pathways that interfere in the same vibrational state. Frequency modulating one of the fields leads to amplitude modulations on all of the fields. This vibrational molecular interferometry (VMI) technique allows imaging at high speed free of non-resonant background, and is able to distinguish between electronic and vibrational contributions to the total signal

KW - METIS-286037

KW - IR-84664

U2 - 10.1117/12.908158

DO - 10.1117/12.908158

M3 - Conference contribution

SN - 9780819488695

T3 - Proceedings of SPIE

BT - Multiphoton Microscopy in the Biomedical Sciences XII

A2 - Periasamy, Ammasi

A2 - König, Karsten

A2 - So, Peter T.C.

PB - SPIE

T2 - SPIE BiOS 2012

Y2 - 21 January 2012 through 26 January 2012

ER -

Garbacik ET, Korterik JP , Otto C, Mukamel S, Herek JL , Offerhaus HL. Background-free nonlinear microspectroscopy with vibrational molecular interferometry. In Periasamy A, König K, So PTC, editors, Multiphoton Microscopy in the Biomedical Sciences XII: 22–24 January 2012, San Francisco, California, United States. SPIE. 2012. 822605. (Proceedings of SPIE). doi: 10.1117/12.908158

Background-free nonlinear microspectroscopy with vibrational molecular interferometry

Abstract

Publication series

Conference

Keywords

Access to Document

Fingerprint

Cite this