Coherent Control of the Exciton Dynamics in the FMO Protein

M.T.W. Milder; B. Brüggemann; M. Miller; J L. Herek

doi:10.1007/978-3-540-95946-5_145

Coherent Control of the Exciton Dynamics in the FMO Protein

M.T.W. Milder^*, B. Brüggemann, M. Miller, J L. Herek

^*Corresponding author for this work

Optical Sciences

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

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Abstract

We have achieved first steps toward coherent control of excitonic energy migration in the FMO pigment-protein complex, by combining femtosecond pulse shaping with a feedback loop using an evolutionary algorithm. The experimental conditions achieved, with a rotating sample, a cryostat, and a pulse shaper, are sufficient for closed loop optimizations.

Original language	English
Title of host publication	Ultrafast Phenomena XVI
Subtitle of host publication	Proceedings of the 16th International Conference, Palazzo dei Congressi Stresa, Italy, June 9-13, 2008
Editors	Paul Corkum, Sandro Silvestri, Keith A. Nelson, Eberhard Riedle, Robert W. Schoenlein
Place of Publication	Berlin, Heidelberg
Publisher	Springer
Pages	448-450
Number of pages	3
ISBN (Electronic)	978-3-540-95946-5
ISBN (Print)	978-3-540-95945-8, 978-3-662-50172-6
DOIs	https://doi.org/10.1007/978-3-540-95946-5_145
Publication status	Published - 2009
Event	16th International Conference on Ultrafast Phenomena 2008 - Stresa, Italy Duration: 9 Jun 2008 → 13 Jun 2008 Conference number: 16

Publication series

Name	Springer Series in Chemical Physics
Publisher	Springer
Volume	92
ISSN (Print)	0172-6218
ISSN (Electronic)	2364-9003

Conference

Conference	16th International Conference on Ultrafast Phenomena 2008
Abbreviated title	Ultrafast Phenomena XVI
City	Stresa, Italy
Period	9/06/08 → 13/06/08

Keywords

Coherent control
Exciton level
Green sulfur bacterium
Linear chirp
Transient absorption spectrum
2023 OA procedure

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10.1007/978-3-540-95946-5_145

ArticleFinal published version, 887 KBLicence: Taverne

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Milder, M. T. W., Brüggemann, B., Miller, M., & Herek, J. L. (2009). Coherent Control of the Exciton Dynamics in the FMO Protein. In P. Corkum, S. Silvestri, K. A. Nelson, E. Riedle, & R. W. Schoenlein (Eds.), Ultrafast Phenomena XVI: Proceedings of the 16th International Conference, Palazzo dei Congressi Stresa, Italy, June 9-13, 2008 (pp. 448-450). (Springer Series in Chemical Physics; Vol. 92). Springer. https://doi.org/10.1007/978-3-540-95946-5_145

Milder, M.T.W. ; Brüggemann, B. ; Miller, M. et al. / Coherent Control of the Exciton Dynamics in the FMO Protein. Ultrafast Phenomena XVI: Proceedings of the 16th International Conference, Palazzo dei Congressi Stresa, Italy, June 9-13, 2008. editor / Paul Corkum ; Sandro Silvestri ; Keith A. Nelson ; Eberhard Riedle ; Robert W. Schoenlein. Berlin, Heidelberg : Springer, 2009. pp. 448-450 (Springer Series in Chemical Physics).

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title = "Coherent Control of the Exciton Dynamics in the FMO Protein",

abstract = "We have achieved first steps toward coherent control of excitonic energy migration in the FMO pigment-protein complex, by combining femtosecond pulse shaping with a feedback loop using an evolutionary algorithm. The experimental conditions achieved, with a rotating sample, a cryostat, and a pulse shaper, are sufficient for closed loop optimizations.",

keywords = "Coherent control, Exciton level, Green sulfur bacterium, Linear chirp, Transient absorption spectrum, 2023 OA procedure",

author = "M.T.W. Milder and B. Br{\"u}ggemann and M. Miller and Herek, {J L.}",

note = "Publisher Copyright: {\textcopyright} 2009, Springer-Verlag Berlin Heidelberg.; 16th International Conference on Ultrafast Phenomena 2008, Ultrafast Phenomena XVI ; Conference date: 09-06-2008 Through 13-06-2008",

year = "2009",

doi = "10.1007/978-3-540-95946-5_145",

language = "English",

isbn = "978-3-540-95945-8",

series = "Springer Series in Chemical Physics",

publisher = "Springer",

pages = "448--450",

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booktitle = "Ultrafast Phenomena XVI",

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Milder, MTW, Brüggemann, B, Miller, M & Herek, JL 2009, Coherent Control of the Exciton Dynamics in the FMO Protein. in P Corkum, S Silvestri, KA Nelson, E Riedle & RW Schoenlein (eds), Ultrafast Phenomena XVI: Proceedings of the 16th International Conference, Palazzo dei Congressi Stresa, Italy, June 9-13, 2008. Springer Series in Chemical Physics, vol. 92, Springer, Berlin, Heidelberg, pp. 448-450, 16th International Conference on Ultrafast Phenomena 2008, Stresa, Italy, 9/06/08. https://doi.org/10.1007/978-3-540-95946-5_145

Coherent Control of the Exciton Dynamics in the FMO Protein. / Milder, M.T.W.; Brüggemann, B.; Miller, M. et al.
Ultrafast Phenomena XVI: Proceedings of the 16th International Conference, Palazzo dei Congressi Stresa, Italy, June 9-13, 2008. ed. / Paul Corkum; Sandro Silvestri; Keith A. Nelson; Eberhard Riedle; Robert W. Schoenlein. Berlin, Heidelberg: Springer, 2009. p. 448-450 (Springer Series in Chemical Physics; Vol. 92).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

TY - GEN

T1 - Coherent Control of the Exciton Dynamics in the FMO Protein

AU - Milder, M.T.W.

AU - Brüggemann, B.

AU - Miller, M.

AU - Herek, J L.

N1 - Conference code: 16

PY - 2009

Y1 - 2009

N2 - We have achieved first steps toward coherent control of excitonic energy migration in the FMO pigment-protein complex, by combining femtosecond pulse shaping with a feedback loop using an evolutionary algorithm. The experimental conditions achieved, with a rotating sample, a cryostat, and a pulse shaper, are sufficient for closed loop optimizations.

AB - We have achieved first steps toward coherent control of excitonic energy migration in the FMO pigment-protein complex, by combining femtosecond pulse shaping with a feedback loop using an evolutionary algorithm. The experimental conditions achieved, with a rotating sample, a cryostat, and a pulse shaper, are sufficient for closed loop optimizations.

KW - Coherent control

KW - Exciton level

KW - Green sulfur bacterium

KW - Linear chirp

KW - Transient absorption spectrum

KW - 2023 OA procedure

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U2 - 10.1007/978-3-540-95946-5_145

DO - 10.1007/978-3-540-95946-5_145

M3 - Conference contribution

AN - SCOPUS:85122398262

SN - 978-3-540-95945-8

SN - 978-3-662-50172-6

T3 - Springer Series in Chemical Physics

SP - 448

EP - 450

BT - Ultrafast Phenomena XVI

A2 - Corkum, Paul

A2 - Silvestri, Sandro

A2 - Nelson, Keith A.

A2 - Riedle, Eberhard

A2 - Schoenlein, Robert W.

PB - Springer

CY - Berlin, Heidelberg

T2 - 16th International Conference on Ultrafast Phenomena 2008

Y2 - 9 June 2008 through 13 June 2008

ER -

Milder MTW, Brüggemann B, Miller M, Herek JL. Coherent Control of the Exciton Dynamics in the FMO Protein. In Corkum P, Silvestri S, Nelson KA, Riedle E, Schoenlein RW, editors, Ultrafast Phenomena XVI: Proceedings of the 16th International Conference, Palazzo dei Congressi Stresa, Italy, June 9-13, 2008. Berlin, Heidelberg: Springer. 2009. p. 448-450. (Springer Series in Chemical Physics). doi: 10.1007/978-3-540-95946-5_145

Coherent Control of the Exciton Dynamics in the FMO Protein

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