Coherent control of two photon fluorescence with a high-resolution spectral phase shaper

S. Postma; Paul Corkum; David M. Jonas; Herman L. Offerhaus; Vinod Subramaniam; R.J.Dwayne Miller; N.F. van Hulst; Andrew M. Weiner

doi:10.1007/978-3-540-68781-8_67

Coherent control of two photon fluorescence with a high-resolution spectral phase shaper

S. Postma, Paul Corkum (Editor), David M. Jonas (Editor), Herman L. Offerhaus, Vinod Subramaniam, R.J.Dwayne Miller (Editor), N.F. van Hulst, Andrew M. Weiner (Editor)

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Abstract

We present effects of spectral shaping on the two-photon fluorescence from fluorescent dye molecules in solution and from quantum dots. The experiments are done with sub-25 fs pulses around 800 nm and a compact (7×10 cm2) high resolution reflective spectral phase shaper. Our results demonstrate that the sign of a phase step in the spectrum of the excitation pulses influences the amount of fluorescence. This implies that beside the two-photon spectral intensity the phase of this spectrum is important as well.

Original language	Undefined
Pages	-
DOIs	https://doi.org/10.1007/978-3-540-68781-8_67
Publication status	Published - 31 Jul 2006

Keywords

IR-72665
METIS-232569

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10.1007/978-3-540-68781-8_67

coherent_control
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Cite this

Postma, S., Corkum, P. (Ed.), Jonas, D. M. (Ed.), Offerhaus, H. L., Subramaniam, V., Miller, R. J. D. (Ed.), ... Weiner, A. M. (Ed.) (2006). Coherent control of two photon fluorescence with a high-resolution spectral phase shaper. -. https://doi.org/10.1007/978-3-540-68781-8_67

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AU - Offerhaus, Herman L.

AU - Subramaniam, Vinod

AU - van Hulst, N.F.

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A2 - Weiner, Andrew M.

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AB - We present effects of spectral shaping on the two-photon fluorescence from fluorescent dye molecules in solution and from quantum dots. The experiments are done with sub-25 fs pulses around 800 nm and a compact (7×10 cm2) high resolution reflective spectral phase shaper. Our results demonstrate that the sign of a phase step in the spectrum of the excitation pulses influences the amount of fluorescence. This implies that beside the two-photon spectral intensity the phase of this spectrum is important as well.

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