Concentration polariztion to measure nano-pore accessibility

Miguel  Solsona; Anne-Eva  Nieuwelink; Vasileios A. Papadimitriou; Jan C.T. Eijkel; Florian Meirer; Leon  Abelmann; Wouter  Olthuis; Bert M. Weckhuysen; Albert  van den Berg

Concentration polariztion to measure nano-pore accessibility

Miguel Solsona, Anne-Eva Nieuwelink, Vasileios A. Papadimitriou, Jan C.T. Eijkel, Florian Meirer, Leon Abelmann, Wouter Olthuis, Bert M. Weckhuysen, Albert van den Berg

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

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Abstract

Understanding the deactivation process in porous catalysts is of tremendous economic significance. We demonstrate the feasibility of using the concentration polarization method to obtain the pore accessibility distribution at single particle level for the first time. By using this technique we could measure the pore blockage caused by Fe in fluid catalytic cracking particles as evidenced by correlating it to the activity. We expect this new single particle technique to increase our understanding of the deactivation processes occurring in porous catalysts.

Original language	English
Title of host publication	21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017
Editors	Abraham Lee, Don DeVoe
Publisher	The Chemical and Biological Microsystems Society
Pages	1497-1498
Number of pages	2
ISBN (Print)	978-0-692-94183-6
Publication status	Published - 22 Oct 2017
Event	21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, μTAS 2017 - Savannah International Trade & Convention Center, Savannah, United States Duration: 22 Oct 2017 → 26 Oct 2017 Conference number: 21 https://www.microtas2017.org/

Publication series

Name	International Conference on Miniaturized Systems for Chemistry and Life Sciences (μTAS)
Publisher	Transducers Research Foundations, Inc.
Volume	2017
ISSN (Print)	1556-5904

Conference

Conference	21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, μTAS 2017
Abbreviated title	MicroTAS
Country/Territory	United States
City	Savannah
Period	22/10/17 → 26/10/17
Internet address	https://www.microtas2017.org/

Keywords

Catalysts
Concentration polarization
Heterogeneous porosity

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Solsona, M., Nieuwelink, A.-E., Papadimitriou, V. A., Eijkel, J. C. T., Meirer, F., Abelmann, L., Olthuis, W., Weckhuysen, B. M., & van den Berg, A. (2017). Concentration polariztion to measure nano-pore accessibility. In A. Lee, & D. DeVoe (Eds.), 21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017 (pp. 1497-1498). (International Conference on Miniaturized Systems for Chemistry and Life Sciences (μTAS); Vol. 2017). The Chemical and Biological Microsystems Society.

Solsona, Miguel ; Nieuwelink, Anne-Eva ; Papadimitriou, Vasileios A. et al. / Concentration polariztion to measure nano-pore accessibility. 21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017. editor / Abraham Lee ; Don DeVoe. The Chemical and Biological Microsystems Society, 2017. pp. 1497-1498 (International Conference on Miniaturized Systems for Chemistry and Life Sciences (μTAS)).

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title = "Concentration polariztion to measure nano-pore accessibility",

abstract = "Understanding the deactivation process in porous catalysts is of tremendous economic significance. We demonstrate the feasibility of using the concentration polarization method to obtain the pore accessibility distribution at single particle level for the first time. By using this technique we could measure the pore blockage caused by Fe in fluid catalytic cracking particles as evidenced by correlating it to the activity. We expect this new single particle technique to increase our understanding of the deactivation processes occurring in porous catalysts.",

keywords = "Catalysts, Concentration polarization, Heterogeneous porosity",

author = "Miguel Solsona and Anne-Eva Nieuwelink and Papadimitriou, {Vasileios A.} and Eijkel, {Jan C.T.} and Florian Meirer and Leon Abelmann and Wouter Olthuis and Weckhuysen, {Bert M.} and {van den Berg}, Albert",

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editor = "Abraham Lee and Don DeVoe",

booktitle = "21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017",

note = "21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, μTAS 2017, MicroTAS ; Conference date: 22-10-2017 Through 26-10-2017",

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Solsona, M, Nieuwelink, A-E, Papadimitriou, VA, Eijkel, JCT, Meirer, F, Abelmann, L, Olthuis, W, Weckhuysen, BM & van den Berg, A 2017, Concentration polariztion to measure nano-pore accessibility. in A Lee & D DeVoe (eds), 21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017. International Conference on Miniaturized Systems for Chemistry and Life Sciences (μTAS), vol. 2017, The Chemical and Biological Microsystems Society, pp. 1497-1498, 21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, μTAS 2017, Savannah, Georgia, United States, 22/10/17.

Concentration polariztion to measure nano-pore accessibility. / Solsona, Miguel ; Nieuwelink, Anne-Eva ; Papadimitriou, Vasileios A. et al.
21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017. ed. / Abraham Lee; Don DeVoe. The Chemical and Biological Microsystems Society, 2017. p. 1497-1498 (International Conference on Miniaturized Systems for Chemistry and Life Sciences (μTAS); Vol. 2017).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

TY - GEN

T1 - Concentration polariztion to measure nano-pore accessibility

AU - Solsona, Miguel

AU - Nieuwelink, Anne-Eva

AU - Papadimitriou, Vasileios A.

AU - Eijkel, Jan C.T.

AU - Meirer, Florian

AU - Abelmann, Leon

AU - Olthuis, Wouter

AU - Weckhuysen, Bert M.

AU - van den Berg, Albert

N1 - Conference code: 21

PY - 2017/10/22

Y1 - 2017/10/22

N2 - Understanding the deactivation process in porous catalysts is of tremendous economic significance. We demonstrate the feasibility of using the concentration polarization method to obtain the pore accessibility distribution at single particle level for the first time. By using this technique we could measure the pore blockage caused by Fe in fluid catalytic cracking particles as evidenced by correlating it to the activity. We expect this new single particle technique to increase our understanding of the deactivation processes occurring in porous catalysts.

AB - Understanding the deactivation process in porous catalysts is of tremendous economic significance. We demonstrate the feasibility of using the concentration polarization method to obtain the pore accessibility distribution at single particle level for the first time. By using this technique we could measure the pore blockage caused by Fe in fluid catalytic cracking particles as evidenced by correlating it to the activity. We expect this new single particle technique to increase our understanding of the deactivation processes occurring in porous catalysts.

KW - Catalysts

KW - Concentration polarization

KW - Heterogeneous porosity

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M3 - Conference contribution

SN - 978-0-692-94183-6

T3 - International Conference on Miniaturized Systems for Chemistry and Life Sciences (μTAS)

SP - 1497

EP - 1498

BT - 21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017

A2 - Lee, Abraham

A2 - DeVoe, Don

PB - The Chemical and Biological Microsystems Society

T2 - 21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, μTAS 2017

Y2 - 22 October 2017 through 26 October 2017

ER -

Solsona M, Nieuwelink AE, Papadimitriou VA, Eijkel JCT, Meirer F, Abelmann L et al. Concentration polariztion to measure nano-pore accessibility. In Lee A, DeVoe D, editors, 21st International Conference on Miniaturized Systems for Chemistry and Life Sciences, MicroTAS 2017. The Chemical and Biological Microsystems Society. 2017. p. 1497-1498. (International Conference on Miniaturized Systems for Chemistry and Life Sciences (μTAS)).

Concentration polariztion to measure nano-pore accessibility

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