Abstract
The nonlinear optical behaviour of a crystalline adlayer of unidirectionally oriented macromolecules at a substrate is studied by means of the discrete dipole model. Polar and azimuthal dependence of the second harmonic pp-reflectance is investigated at the fundamental and second harmonic frequencies. The influence of the anisotropic linear properties of the adlayer turns out to be essential.
| Original language | English |
|---|---|
| Pages (from-to) | 7767-7770 |
| Number of pages | 4 |
| Journal | Physical Review B (Condensed Matter) |
| Volume | 152 |
| Issue number | 1 |
| DOIs | |
| Publication status | Published - 1995 |