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Deeper mechanistic insights into epitaxial nickelate electrocatalysts for the oxygen evolution reaction

  • Ellen M. Kiens
  • , Min Ju Choi
  • , Luhan Wei
  • , Qiyang Lu
  • , Le Wang
  • , Christoph Baeumer*
  • *Corresponding author for this work

Research output: Contribution to journalArticleAcademicpeer-review

198 Downloads (Pure)

Abstract

Mass production of green hydrogen via water electrolysis requires advancements in the performance of electrocatalysts, especially for the oxygen evolution reaction. In this feature article, we highlight how epitaxial nickelates act as model systems to identify atomic-level composition-structure-property-activity relationships, capture dynamic changes under operating conditions, and reveal reaction and failure mechanisms. These insights guide advanced electrocatalyst design with tailored functionality and superior performance. We conclude with an outlook for future developments via operando characterization and multilayer electrocatalyst design.

Original languageEnglish
Pages (from-to)4562-4577
Number of pages16
JournalChemical communications
Volume59
Issue number31
DOIs
Publication statusPublished - 2 Mar 2023

Keywords

  • UT-Hybrid-D

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