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Elastocapillary levelling of thin viscous films on soft substrates

  • Marco Rivetti
  • , Vincent Luc Bertin
  • , Thomas Salez
  • , Chung-Yuen Hui
  • , Christine Linne
  • , Maxence Arutkin
  • , Haibin Wu
  • , Elie Raphaël
  • , Oliver Bäumchen*
  • *Corresponding author for this work

Research output: Contribution to journalArticleAcademicpeer-review

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Abstract

A thin liquid film with nonzero curvature at its free surface spontaneously flows to reach a flat configuration, a process driven by Laplace pressure gradients and resisted by the liquid's viscosity. Inspired by recent progresses on the dynamics of liquid droplets on soft substrates, we here study the relaxation of a viscous film supported by an elastic foundation. Experiments involve thin polymer films on elastomeric substrates, where the dynamics of the liquid-air interface is monitored using atomic force microscopy. A theoretical model that describes the coupled evolution of the solid-liquid and the liquid-air interfaces is also provided. In this soft-levelling configuration, Laplace pressure gradients not only drive the flow, but they also induce elastic deformations on the substrate that affect the flow and the shape of the liquid-air interface itself. This process represents an original example of elastocapillarity that is not mediated by the presence of a contact line. We discuss the impact of the elastic contribution on the levelling dynamics and show the departure from the classical self-similarities and power laws observed for capillary levelling on rigid substrates.
Original languageEnglish
Article number094001
JournalPhysical review fluids
Volume2
Issue number9
DOIs
Publication statusPublished - 1 Sept 2017
Externally publishedYes

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