Experimental validation of packed bed chemical-looping combustion

S. Noorman, M. van Sint Annaland, J.A.M. Kuipers

    Research output: Contribution to journalArticleAcademic

    67 Citations (Scopus)

    Abstract

    Chemical-looping combustion has emerged as a promising alternative technology, intrinsically integrating CO2 capture in power production. A novel reactor concept based on dynamically operated packed beds has been proposed [Noorman, S., van Sint Annaland, M., Kuipers, J.A.M., 2007. Packed bed reactor technology for chemical-looping combustion. Ind. Eng. Chem. Res. 46, 4212–4220] and in this work, packed bed chemical-looping combustion was investigated experimentally to provide an experimental proof-of-principle. Using information obtained from both the reduction and oxidation cycles, the measured maximum temperature rise and front velocities in the packed bed during the oxidation cycle corresponded very well with analytical expressions describing the system, especially when the contribution of the formation of carbon during the reduction cycle was taken into account.
    Original languageUndefined
    Pages (from-to)92-97
    JournalChemical engineering science
    Volume65
    Issue number1
    DOIs
    Publication statusPublished - 2010

    Keywords

    • IR-70210

    Cite this

    Noorman, S. ; van Sint Annaland, M. ; Kuipers, J.A.M. / Experimental validation of packed bed chemical-looping combustion. In: Chemical engineering science. 2010 ; Vol. 65, No. 1. pp. 92-97.
    @article{16c4b8bcdabb42c2acb372487afcb38a,
    title = "Experimental validation of packed bed chemical-looping combustion",
    abstract = "Chemical-looping combustion has emerged as a promising alternative technology, intrinsically integrating CO2 capture in power production. A novel reactor concept based on dynamically operated packed beds has been proposed [Noorman, S., van Sint Annaland, M., Kuipers, J.A.M., 2007. Packed bed reactor technology for chemical-looping combustion. Ind. Eng. Chem. Res. 46, 4212–4220] and in this work, packed bed chemical-looping combustion was investigated experimentally to provide an experimental proof-of-principle. Using information obtained from both the reduction and oxidation cycles, the measured maximum temperature rise and front velocities in the packed bed during the oxidation cycle corresponded very well with analytical expressions describing the system, especially when the contribution of the formation of carbon during the reduction cycle was taken into account.",
    keywords = "IR-70210",
    author = "S. Noorman and {van Sint Annaland}, M. and J.A.M. Kuipers",
    year = "2010",
    doi = "10.1016/j.ces.2009.02.004",
    language = "Undefined",
    volume = "65",
    pages = "92--97",
    journal = "Chemical engineering science",
    issn = "0009-2509",
    publisher = "Elsevier",
    number = "1",

    }

    Experimental validation of packed bed chemical-looping combustion. / Noorman, S.; van Sint Annaland, M.; Kuipers, J.A.M.

    In: Chemical engineering science, Vol. 65, No. 1, 2010, p. 92-97.

    Research output: Contribution to journalArticleAcademic

    TY - JOUR

    T1 - Experimental validation of packed bed chemical-looping combustion

    AU - Noorman, S.

    AU - van Sint Annaland, M.

    AU - Kuipers, J.A.M.

    PY - 2010

    Y1 - 2010

    N2 - Chemical-looping combustion has emerged as a promising alternative technology, intrinsically integrating CO2 capture in power production. A novel reactor concept based on dynamically operated packed beds has been proposed [Noorman, S., van Sint Annaland, M., Kuipers, J.A.M., 2007. Packed bed reactor technology for chemical-looping combustion. Ind. Eng. Chem. Res. 46, 4212–4220] and in this work, packed bed chemical-looping combustion was investigated experimentally to provide an experimental proof-of-principle. Using information obtained from both the reduction and oxidation cycles, the measured maximum temperature rise and front velocities in the packed bed during the oxidation cycle corresponded very well with analytical expressions describing the system, especially when the contribution of the formation of carbon during the reduction cycle was taken into account.

    AB - Chemical-looping combustion has emerged as a promising alternative technology, intrinsically integrating CO2 capture in power production. A novel reactor concept based on dynamically operated packed beds has been proposed [Noorman, S., van Sint Annaland, M., Kuipers, J.A.M., 2007. Packed bed reactor technology for chemical-looping combustion. Ind. Eng. Chem. Res. 46, 4212–4220] and in this work, packed bed chemical-looping combustion was investigated experimentally to provide an experimental proof-of-principle. Using information obtained from both the reduction and oxidation cycles, the measured maximum temperature rise and front velocities in the packed bed during the oxidation cycle corresponded very well with analytical expressions describing the system, especially when the contribution of the formation of carbon during the reduction cycle was taken into account.

    KW - IR-70210

    U2 - 10.1016/j.ces.2009.02.004

    DO - 10.1016/j.ces.2009.02.004

    M3 - Article

    VL - 65

    SP - 92

    EP - 97

    JO - Chemical engineering science

    JF - Chemical engineering science

    SN - 0009-2509

    IS - 1

    ER -