TY - JOUR
T1 - Few-emitter lasing in single ultra-small nanocavities
AU - Ojambati, Oluwafemi S.
AU - Arnardóttir, Kristín B.
AU - Lovett, Brendon W.
AU - Keeling, Jonathan
AU - Baumberg, Jeremy J.
N1 - Publisher Copyright:
© 2024 the author(s), published by De Gruyter, Berlin/Boston 2024.
PY - 2024/6
Y1 - 2024/6
N2 - Lasers are ubiquitous for information storage, processing, communications, sensing, biological research and medical applications. To decrease their energy and materials usage, a key quest is to miniaturise lasers down to nanocavities. Obtaining the smallest mode volumes demands plasmonic nanocavities, but for these, gain comes from only a single or few emitters. Until now, lasing in such devices was unobtainable due to low gain and high cavity losses. Here, we demonstrate a form of 'few emitter lasing' in a plasmonic nanocavity approaching the single-molecule emitter regime. The few-emitter lasing transition significantly broadens, and depends on the number of molecules and their individual locations. We show this non-standard few-emitter lasing can be understood by developing a theoretical approach extending previous weak-coupling theories. Our work paves the way for developing nanolaser applications as well as fundamental studies at the limit of few emitters.
AB - Lasers are ubiquitous for information storage, processing, communications, sensing, biological research and medical applications. To decrease their energy and materials usage, a key quest is to miniaturise lasers down to nanocavities. Obtaining the smallest mode volumes demands plasmonic nanocavities, but for these, gain comes from only a single or few emitters. Until now, lasing in such devices was unobtainable due to low gain and high cavity losses. Here, we demonstrate a form of 'few emitter lasing' in a plasmonic nanocavity approaching the single-molecule emitter regime. The few-emitter lasing transition significantly broadens, and depends on the number of molecules and their individual locations. We show this non-standard few-emitter lasing can be understood by developing a theoretical approach extending previous weak-coupling theories. Our work paves the way for developing nanolaser applications as well as fundamental studies at the limit of few emitters.
KW - emitter
KW - nanocavity
KW - nanolaser
KW - nonlinear light emission
KW - plasmonic nanocavity
UR - http://www.scopus.com/inward/record.url?scp=85182886894&partnerID=8YFLogxK
U2 - 10.1515/nanoph-2023-0706
DO - 10.1515/nanoph-2023-0706
M3 - Article
AN - SCOPUS:85182886894
SN - 2192-8606
SN - 2192-8614
VL - 13
SP - 2679
EP - 2686
JO - Nanophotonics
JF - Nanophotonics
IS - 14
ER -