Highly ordered C60 films on epitaxial Fe/MgO(001) surfaces for organic spintronics

P.K.J. Wong, T. Lan Ahn Tran, Peter Brinks, Wilfred Gerard van der Wiel, Mark Huijben, Machiel Pieter de Jong

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Abstract

Hybrid interfaces between ferromagnetic surfaces and carbon-based molecules play an important role in organic spintronics. The fabrication of devices with well defined interfaces remains challenging, however, hampering microscopic understanding of their operation mechanisms. We have studied the crystallinity and molecular ordering of C-60 films on epitaxial Fe/MgO(001) surfaces, using X-ray diffraction and scanning tunneling microscopy (STM). Both techniques confirm that fcc molecular C-60 films with a (111)-texture can be fabricated on epitaxial bcc-Fe(001) surfaces at elevated growth temperatures (100-130 degrees C). STM measurements show that C-60 monolayers deposited at 130 degrees C are highly ordered, exhibiting quasi-hexagonal arrangements on the Fe(001) surface oriented along the [100] and [010] directions. The mismatch between the surface lattice of the monolayer and the bulk fcc C-60 lattice prevents epitaxial overgrowth of multilayers. (C) 2012 Elsevier B.V. All rights reserved.
Original languageUndefined
Pages (from-to)451-456
Number of pages6
JournalOrganic electronics
Volume14
Issue number2
DOIs
Publication statusPublished - Feb 2013

Keywords

  • METIS-295997
  • IR-89200
  • EWI-24404

Cite this

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title = "Highly ordered C60 films on epitaxial Fe/MgO(001) surfaces for organic spintronics",
abstract = "Hybrid interfaces between ferromagnetic surfaces and carbon-based molecules play an important role in organic spintronics. The fabrication of devices with well defined interfaces remains challenging, however, hampering microscopic understanding of their operation mechanisms. We have studied the crystallinity and molecular ordering of C-60 films on epitaxial Fe/MgO(001) surfaces, using X-ray diffraction and scanning tunneling microscopy (STM). Both techniques confirm that fcc molecular C-60 films with a (111)-texture can be fabricated on epitaxial bcc-Fe(001) surfaces at elevated growth temperatures (100-130 degrees C). STM measurements show that C-60 monolayers deposited at 130 degrees C are highly ordered, exhibiting quasi-hexagonal arrangements on the Fe(001) surface oriented along the [100] and [010] directions. The mismatch between the surface lattice of the monolayer and the bulk fcc C-60 lattice prevents epitaxial overgrowth of multilayers. (C) 2012 Elsevier B.V. All rights reserved.",
keywords = "METIS-295997, IR-89200, EWI-24404",
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year = "2013",
month = "2",
doi = "10.1016/j.orgel.2012.11.034",
language = "Undefined",
volume = "14",
pages = "451--456",
journal = "Organic electronics",
issn = "1566-1199",
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Highly ordered C60 films on epitaxial Fe/MgO(001) surfaces for organic spintronics. / Wong, P.K.J.; Tran, T. Lan Ahn; Brinks, Peter; van der Wiel, Wilfred Gerard; Huijben, Mark; de Jong, Machiel Pieter.

In: Organic electronics, Vol. 14, No. 2, 02.2013, p. 451-456.

Research output: Contribution to journalArticleAcademicpeer-review

TY - JOUR

T1 - Highly ordered C60 films on epitaxial Fe/MgO(001) surfaces for organic spintronics

AU - Wong, P.K.J.

AU - Tran, T. Lan Ahn

AU - Brinks, Peter

AU - van der Wiel, Wilfred Gerard

AU - Huijben, Mark

AU - de Jong, Machiel Pieter

PY - 2013/2

Y1 - 2013/2

N2 - Hybrid interfaces between ferromagnetic surfaces and carbon-based molecules play an important role in organic spintronics. The fabrication of devices with well defined interfaces remains challenging, however, hampering microscopic understanding of their operation mechanisms. We have studied the crystallinity and molecular ordering of C-60 films on epitaxial Fe/MgO(001) surfaces, using X-ray diffraction and scanning tunneling microscopy (STM). Both techniques confirm that fcc molecular C-60 films with a (111)-texture can be fabricated on epitaxial bcc-Fe(001) surfaces at elevated growth temperatures (100-130 degrees C). STM measurements show that C-60 monolayers deposited at 130 degrees C are highly ordered, exhibiting quasi-hexagonal arrangements on the Fe(001) surface oriented along the [100] and [010] directions. The mismatch between the surface lattice of the monolayer and the bulk fcc C-60 lattice prevents epitaxial overgrowth of multilayers. (C) 2012 Elsevier B.V. All rights reserved.

AB - Hybrid interfaces between ferromagnetic surfaces and carbon-based molecules play an important role in organic spintronics. The fabrication of devices with well defined interfaces remains challenging, however, hampering microscopic understanding of their operation mechanisms. We have studied the crystallinity and molecular ordering of C-60 films on epitaxial Fe/MgO(001) surfaces, using X-ray diffraction and scanning tunneling microscopy (STM). Both techniques confirm that fcc molecular C-60 films with a (111)-texture can be fabricated on epitaxial bcc-Fe(001) surfaces at elevated growth temperatures (100-130 degrees C). STM measurements show that C-60 monolayers deposited at 130 degrees C are highly ordered, exhibiting quasi-hexagonal arrangements on the Fe(001) surface oriented along the [100] and [010] directions. The mismatch between the surface lattice of the monolayer and the bulk fcc C-60 lattice prevents epitaxial overgrowth of multilayers. (C) 2012 Elsevier B.V. All rights reserved.

KW - METIS-295997

KW - IR-89200

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JO - Organic electronics

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SN - 1566-1199

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