Influence of Bubbles on the Energy Conversion Efficiency of Electrochemical Reactors

Andrea Angulo; Peter van der Linde; Han Gardeniers; Miguel Modestino; David Fernández Rivas

doi:10.48550/arXiv.2002.08167

Influence of Bubbles on the Energy Conversion Efficiency of Electrochemical Reactors

Andrea Angulo
, Peter van der Linde
, Han Gardeniers
, Miguel Modestino
, David Fernández Rivas

Research output: Working paper › Preprint › Academic

51 Downloads (Pure)

Abstract

Bubbles are known to influence energy and mass transfer in gas evolving electrodes. However, we lack a detailed understanding on the intricate dependencies between bubble evolution processes and electrochemical phenomena. This review discusses our current knowledge on the effects of bubbles on electrochemical systems with the aim to identify opportunities and motivate future research in this area. We first provide a base background on the physics of bubble evolution as it relates to electrochemical processes. Then we outline how bubbles affect energy efficiency of electrode processes, detailing the bubble-induced impacts on activation, ohmic and concentration overpotentials. Lastly, we describe different strategies to mitigate losses and how to exploit bubbles to enhance electrochemical reactions.

Original language	English
Publisher	ArXiv.org
DOIs	https://doi.org/10.48550/arXiv.2002.08167
Publication status	Published - 12 Feb 2020

Keywords

cond-mat.soft
physics.flu-dyn

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10.48550/arXiv.2002.08167

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1 Review article

Influence of Bubbles on the Energy Conversion Efficiency of Electrochemical Reactors
Angulo, A., van der Linde, P., Gardeniers, H., Modestino, M. A. & Fernandez Rivas, D., 18 Mar 2020, In: Joule. 4, 3, p. 555-579 25 p.
Research output: Contribution to journal › Review article › Academic › peer-review

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Cite this

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abstract = " Bubbles are known to influence energy and mass transfer in gas evolving electrodes. However, we lack a detailed understanding on the intricate dependencies between bubble evolution processes and electrochemical phenomena. This review discusses our current knowledge on the effects of bubbles on electrochemical systems with the aim to identify opportunities and motivate future research in this area. We first provide a base background on the physics of bubble evolution as it relates to electrochemical processes. Then we outline how bubbles affect energy efficiency of electrode processes, detailing the bubble-induced impacts on activation, ohmic and concentration overpotentials. Lastly, we describe different strategies to mitigate losses and how to exploit bubbles to enhance electrochemical reactions. ",

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AU - van der Linde, Peter

AU - Gardeniers, Han

AU - Modestino, Miguel

AU - Rivas, David Fernández

N1 - Joule(2020)

PY - 2020/2/12

Y1 - 2020/2/12

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KW - physics.flu-dyn

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BT - Influence of Bubbles on the Energy Conversion Efficiency of Electrochemical Reactors

PB - ArXiv.org

ER -

Influence of Bubbles on the Energy Conversion Efficiency of Electrochemical Reactors

Abstract

Keywords

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Influence of Bubbles on the Energy Conversion Efficiency of Electrochemical Reactors

Cite this