Magnetic interlayer exchange coupling in epitaxial Fe/Si/Fe (001) studied by polarized neutron reflectometry

R. W. van de Kruijs, M. Th Rekveldt, H. Fredrikze, J. T. Kohlhepp, J. K. Ha, W. J. de Jonge

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Abstract

Polarized neutron reflectometry (PNR) has been used to investigate the magnetic interlayer coupling in a MBE-grown Fe/Si/Fe(001) sandwich at room temperature and at 10 K. Both the magnitude and orientation of the magnetic moments of the Fe layers are obtained from a rigorous analysis of the PNR data. Orthogonal configurations of the Fe magnetizations were observed, providing unambiguous evidence for the presence of a biquadratic term in the exchange coupling energy. The competition between the bilinear and biquadratic exchange couplings results in distinct orthogonal and antiparallel configurations of the Fe magnetizations at room temperature. A previously unresolved magnetic configuration in the room-temperature hysteresis curve was identified by the PNR measurements as a 180° spin-flop transition. The dominant role of the biquadratic coupling at low temperatures is evident from the orthogonal configuration of the magnetizations at remanence in the measurements at T = 10 K. The magnetic configurations deduced by PNR are in good agreement with those obtained by fitting the magnetic hysteresis loops using a global energy minimum calculation.

Original languageEnglish
Article number064440
Pages (from-to)644401-644407
Number of pages7
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume65
Issue number6
Early online date24 Jan 2002
DOIs
Publication statusPublished - 1 Feb 2002
Externally publishedYes

Keywords

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