Nanophotonic control of the Forster resonance energy transfer efficiency

Christian Blum, Niels Zijlstra, Ad Lagendijk, Martijn Wubs, Allard P. Mosk, Vinod Subramaniam, Willem L. Vos

Research output: Contribution to journalArticleAcademicpeer-review

106 Citations (Scopus)
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Abstract

We have studied the influence of the local density of optical states (LDOS) on the rate and efficiency of Förster resonance energy transfer (FRET) from a donor to an acceptor. The donors and acceptors are dye molecules that are separated by a short strand of double-stranded DNA. The LDOS is controlled by carefully positioning the FRET pairs near a mirror. We find that the energy transfer efficiency changes with LDOS, and that, in agreement with theory, the energy transfer rate is independent of the LDOS, which allows one to quantitatively control FRET systems in a new way. Our results imply a change in the characteristic Förster distance, in contrast to common lore that this distance is fixed for a given FRET pair
Original languageEnglish
Article number203601
Number of pages5
JournalPhysical review letters
Volume109
Issue number20
DOIs
Publication statusPublished - 2012

Keywords

  • METIS-289436
  • IR-84731

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