TY - UNPB
T1 - Observation of Mermin-Wagner behavior in LaFeO$_3$/SrTiO$_3$ superlattices
AU - Kiaba, Michal
AU - Suter, Andreas
AU - Salman, Zaher
AU - Prokscha, Thomas
AU - Chen, Binbin
AU - Koster, Gertjan
AU - Dubroka, Adam
PY - 2024/5/7
Y1 - 2024/5/7
N2 - Two-dimensional magnetic materials attract a lot of attention since they potentially exhibit new magnetic properties due to, e.g., strongly enhanced spin fluctuations. However, the suppression of the long-range magnetic order in two dimensions due to long-wavelength spin fluctuations, as suggested by the Mermin-Wagner theorem, has been questioned for finite-size laboratory samples. Here we study the magnetic properties of a dimensional crossover in superlattices composed of the antiferromagnetic LaFeO$_3$ and SrTiO$_3$ that, thanks to their large lateral size, allowed examination using a sensitive magnetic probe - muon spin rotation spectroscopy. We show that the iron electronic moments in superlattices with 3 and 2 monolayers of LaFeO$_3$ exhibit a static antiferromagnetic order. In contrast, in the superlattices with single LaFeO$_3$ monolayer, the moments do not order and fluctuate to the lowest measured temperature as expected from the Mermin-Wagner theorem. Our work shows how dimensionality can be used to tune the magnetic properties of ultrathin films.
AB - Two-dimensional magnetic materials attract a lot of attention since they potentially exhibit new magnetic properties due to, e.g., strongly enhanced spin fluctuations. However, the suppression of the long-range magnetic order in two dimensions due to long-wavelength spin fluctuations, as suggested by the Mermin-Wagner theorem, has been questioned for finite-size laboratory samples. Here we study the magnetic properties of a dimensional crossover in superlattices composed of the antiferromagnetic LaFeO$_3$ and SrTiO$_3$ that, thanks to their large lateral size, allowed examination using a sensitive magnetic probe - muon spin rotation spectroscopy. We show that the iron electronic moments in superlattices with 3 and 2 monolayers of LaFeO$_3$ exhibit a static antiferromagnetic order. In contrast, in the superlattices with single LaFeO$_3$ monolayer, the moments do not order and fluctuate to the lowest measured temperature as expected from the Mermin-Wagner theorem. Our work shows how dimensionality can be used to tune the magnetic properties of ultrathin films.
KW - cond-mat.str-el
KW - cond-mat.mtrl-sci
U2 - 10.48550/arXiv.2405.04293
DO - 10.48550/arXiv.2405.04293
M3 - Preprint
BT - Observation of Mermin-Wagner behavior in LaFeO$_3$/SrTiO$_3$ superlattices
PB - ArXiv.org
ER -