Oxidative coupling of methane over doped Li/MgO catalysts

G.C. Hoogendam; K. Seshan; J.G. van Ommen; J.R.H. Ross

doi:10.1016/0920-5861(94)80154-1

Oxidative coupling of methane over doped Li/MgO catalysts

G.C. Hoogendam^*, K. Seshan, J.G. van Ommen, J.R.H. Ross

^*Corresponding author for this work

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Abstract

A series of zirconia doped Li/MgO catalysts with a fixed amount of zirconia and varying concentrations of lithium was used for the oxidative coupling of methane. It was found that an increase in lithium concentration resulted in a decrease in initial activity, while the selectivity was not affected. The life-time of Zr doped Li/MgO catalysts with a fixed concentration of ZrO2 is a function of the lithium concentration. Previous results have shown that Li2Mg3ZrO6 is active and selective but it is now shown to be instable under reaction conditions.

Original language	English
Pages (from-to)	333-340
Number of pages	8
Journal	Catalysis today
Volume	21
Issue number	2-3
DOIs	https://doi.org/10.1016/0920-5861(94)80154-1
Publication status	Published - 1994

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title = "Oxidative coupling of methane over doped Li/MgO catalysts",

abstract = "A series of zirconia doped Li/MgO catalysts with a fixed amount of zirconia and varying concentrations of lithium was used for the oxidative coupling of methane. It was found that an increase in lithium concentration resulted in a decrease in initial activity, while the selectivity was not affected. The life-time of Zr doped Li/MgO catalysts with a fixed concentration of ZrO2 is a function of the lithium concentration. Previous results have shown that Li2Mg3ZrO6 is active and selective but it is now shown to be instable under reaction conditions.",

author = "G.C. Hoogendam and K. Seshan and {van Ommen}, J.G. and J.R.H. Ross",

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AB - A series of zirconia doped Li/MgO catalysts with a fixed amount of zirconia and varying concentrations of lithium was used for the oxidative coupling of methane. It was found that an increase in lithium concentration resulted in a decrease in initial activity, while the selectivity was not affected. The life-time of Zr doped Li/MgO catalysts with a fixed concentration of ZrO2 is a function of the lithium concentration. Previous results have shown that Li2Mg3ZrO6 is active and selective but it is now shown to be instable under reaction conditions.

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DO - 10.1016/0920-5861(94)80154-1

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VL - 21

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JO - Catalysis today

JF - Catalysis today

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Oxidative coupling of methane over doped Li/MgO catalysts

Abstract

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