Plasma-driven dissociation of CO2 for fuel synthesis

Waldo Bongers (Corresponding Author), Henricus J.M. Bouwmeester, Bram Wolf, Floran Peeters, Stefan Welzel, Dirk van den Bekerom, Niek den Harder, Adelbert Goede, Martijn Graswinckel, Pieter Willem Groen, Jochen Kopecki, Martina Leins, Gerard van Rooij, Andreas Schulz, Matthias Walker, Richard van de Sanden

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68 Citations (Scopus)

Abstract

Power-to-gas is a storage technology aiming to convert surplus electricity from renewable energy sources like wind and solar power into gaseous fuels compatible with the current network infrastructure. Results of CO2 dissociation in a vortexstabilized microwave plasma reactor are presented. The microwave field, residence time, quenching, and vortex configuration were varied to investigate their influence on energy- and conversion efficiency of CO2 dissociation. Significant deterioration of the energy efficiency is observed at forward vortex plasmas upon increasing pressure in the range of 100 mbar towards atmospheric pressure, which is mitigated by using a reverse vortex flow configuration of the plasma reactor. Data from optical emission shows that under all conditions covered by the experiments the gas temperature is in excess of 4000 K, suggesting a predominant thermal dissociation. Different strategies are proposed to enhance energy and conversion efficiencies of plasma-driven dissociation of CO2.
Original languageEnglish
Article number1600126
JournalPlasma processes and polymers
Volume14
Issue number6
DOIs
Publication statusPublished - Jun 2017

Keywords

  • METIS-321259
  • IR-103421

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    Bongers, W., Bouwmeester, H. J. M., Wolf, B., Peeters, F., Welzel, S., van den Bekerom, D., ... van de Sanden, R. (2017). Plasma-driven dissociation of CO2 for fuel synthesis. Plasma processes and polymers, 14(6), [1600126]. https://doi.org/10.1002/ppap.201600126