Single Light Emitters in Electrospun Polymer Nanofibers: Effect of Local Confinement on Radiative Decay

Nikodem Tomczak; Shuying Gu; Mingyong Han; Niek F. van Hulst; G. Julius Vancso

doi:10.1016/j.eurpolymj.2006.06.017

Single Light Emitters in Electrospun Polymer Nanofibers: Effect of Local Confinement on Radiative Decay

Nikodem Tomczak, Shuying Gu, Mingyong Han, Niek F. van Hulst, G. Julius Vancso

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Abstract

The fabrication of light emitting polymer nanofibers by electrospinning of polymer solutions containing either fluorescent organic dye molecules or luminescent semiconductor nanoparticles (quantum dots) is presented. The fluorescence spectra and lifetime of the embedded emitters, down to the level of single molecules were investigated. While the average fluorescence lifetime of single molecules embedded in poly(methyl methacrylate) fibers appears independent of the fiber diameter, the single molecule approach reveals a significant broadening of the fluorescence lifetime distribution for fibers with diameters below the wavelength of light.

Original language	English
Pages (from-to)	2205-2210
Number of pages	6
Journal	European polymer journal
Volume	42
Issue number	10
DOIs	https://doi.org/10.1016/j.eurpolymj.2006.06.017
Publication status	Published - 2006

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title = "Single Light Emitters in Electrospun Polymer Nanofibers: Effect of Local Confinement on Radiative Decay",

abstract = "The fabrication of light emitting polymer nanofibers by electrospinning of polymer solutions containing either fluorescent organic dye molecules or luminescent semiconductor nanoparticles (quantum dots) is presented. The fluorescence spectra and lifetime of the embedded emitters, down to the level of single molecules were investigated. While the average fluorescence lifetime of single molecules embedded in poly(methyl methacrylate) fibers appears independent of the fiber diameter, the single molecule approach reveals a significant broadening of the fluorescence lifetime distribution for fibers with diameters below the wavelength of light.",

author = "Nikodem Tomczak and Shuying Gu and Mingyong Han and {van Hulst}, {Niek F.} and Vancso, {G. Julius}",

year = "2006",

doi = "10.1016/j.eurpolymj.2006.06.017",

language = "English",

volume = "42",

pages = "2205--2210",

journal = "European polymer journal",

issn = "0014-3057",

publisher = "Elsevier Ltd",

number = "10",

}

TY - JOUR

T1 - Single Light Emitters in Electrospun Polymer Nanofibers

T2 - Effect of Local Confinement on Radiative Decay

AU - Tomczak, Nikodem

AU - Gu, Shuying

AU - Han, Mingyong

AU - van Hulst, Niek F.

AU - Vancso, G. Julius

PY - 2006

Y1 - 2006

N2 - The fabrication of light emitting polymer nanofibers by electrospinning of polymer solutions containing either fluorescent organic dye molecules or luminescent semiconductor nanoparticles (quantum dots) is presented. The fluorescence spectra and lifetime of the embedded emitters, down to the level of single molecules were investigated. While the average fluorescence lifetime of single molecules embedded in poly(methyl methacrylate) fibers appears independent of the fiber diameter, the single molecule approach reveals a significant broadening of the fluorescence lifetime distribution for fibers with diameters below the wavelength of light.

AB - The fabrication of light emitting polymer nanofibers by electrospinning of polymer solutions containing either fluorescent organic dye molecules or luminescent semiconductor nanoparticles (quantum dots) is presented. The fluorescence spectra and lifetime of the embedded emitters, down to the level of single molecules were investigated. While the average fluorescence lifetime of single molecules embedded in poly(methyl methacrylate) fibers appears independent of the fiber diameter, the single molecule approach reveals a significant broadening of the fluorescence lifetime distribution for fibers with diameters below the wavelength of light.

U2 - 10.1016/j.eurpolymj.2006.06.017

DO - 10.1016/j.eurpolymj.2006.06.017

M3 - Article

SN - 0014-3057

VL - 42

SP - 2205

EP - 2210

JO - European polymer journal

JF - European polymer journal

IS - 10

ER -

Single Light Emitters in Electrospun Polymer Nanofibers: Effect of Local Confinement on Radiative Decay

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