Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1

A.C.W. van Rhijn; S. Postma; Jeroen P. Korterik; Jennifer Lynn Herek; Herman L. Offerhaus

doi:10.1117/12.808792

Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1

A.C.W. van Rhijn, S. Postma, Jeroen P. Korterik, Jennifer Lynn Herek, Herman L. Offerhaus

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

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Abstract

By spectral phase shaping of both the pump and probe pulses in coherent anti-Stokes Raman scattering (CARS) spectroscopy we demonstrate the extraction of the frequencies of vibrational lines using an unamplified oscillator. Furthermore we demonstrate chemically selective broadband CARS microscopy on a mixed sample of 4 μm diameter polystyrene (PS) and poly(methyl methacrylate) (PMMA) beads. The CARS signal from either the PS or the PMMA beads is shown to be enhanced or suppressed, depending on the phase profile applied to the broadband spectrum. Using a combination of negative and positive (sloped) π-phase steps in the pump and probe spectrum the purely non-resonant background signal is removed

Original language	English
Title of host publication	Multiphoton Microscopy in the Biomedical Sciences IX
Subtitle of host publication	25–27 January 2009, San Jose, California, United States
Editors	Ammasi Periasamy, Peter T.C. So
Place of Publication	Bellingham, WA
Publisher	SPIE
ISBN (Print)	9780819474292
DOIs	https://doi.org/10.1117/12.808792
Publication status	Published - 2009
Event	SPIE International Symposium on Biomedical Optics, BIOS 2009 - San Jose, United States Duration: 24 Jan 2009 → 29 Jan 2009

Publication series

Name	Proceedings of SPIE
Publisher	SPIE
Volume	7183
ISSN (Print)	1605-7422

Conference

Conference	SPIE International Symposium on Biomedical Optics, BIOS 2009
Country/Territory	United States
City	San Jose
Period	24/01/09 → 29/01/09

Keywords

METIS-259553
Non-linear microscopy
Ultrafast spectroscopy
Coherent anti-Stokes Raman scattering
IR-77975

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10.1117/12.808792

Cite this

van Rhijn, A. C. W., Postma, S., Korterik, J. P., Herek, J. L., & Offerhaus, H. L. (2009). Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1. In A. Periasamy, & P. T. C. So (Eds.), Multiphoton Microscopy in the Biomedical Sciences IX: 25–27 January 2009, San Jose, California, United States Article 71830X (Proceedings of SPIE; Vol. 7183). SPIE. https://doi.org/10.1117/12.808792

@inproceedings{52989795f9ef425e82418bf4e2b0554d,

title = "Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1",

abstract = "By spectral phase shaping of both the pump and probe pulses in coherent anti-Stokes Raman scattering (CARS) spectroscopy we demonstrate the extraction of the frequencies of vibrational lines using an unamplified oscillator. Furthermore we demonstrate chemically selective broadband CARS microscopy on a mixed sample of 4 μm diameter polystyrene (PS) and poly(methyl methacrylate) (PMMA) beads. The CARS signal from either the PS or the PMMA beads is shown to be enhanced or suppressed, depending on the phase profile applied to the broadband spectrum. Using a combination of negative and positive (sloped) π-phase steps in the pump and probe spectrum the purely non-resonant background signal is removed",

keywords = "METIS-259553, Non-linear microscopy, Ultrafast spectroscopy, Coherent anti-Stokes Raman scattering, IR-77975",

author = "{van Rhijn}, A.C.W. and S. Postma and Korterik, {Jeroen P.} and Herek, {Jennifer Lynn} and Offerhaus, {Herman L.}",

year = "2009",

doi = "10.1117/12.808792",

language = "English",

isbn = "9780819474292",

series = "Proceedings of SPIE",

publisher = "SPIE",

editor = "Ammasi Periasamy and So, {Peter T.C.}",

booktitle = "Multiphoton Microscopy in the Biomedical Sciences IX",

address = "United States",

note = "SPIE International Symposium on Biomedical Optics, BIOS 2009 ; Conference date: 24-01-2009 Through 29-01-2009",

}

van Rhijn, ACW, Postma, S, Korterik, JP , Herek, JL & Offerhaus, HL 2009, Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1. in A Periasamy & PTC So (eds), Multiphoton Microscopy in the Biomedical Sciences IX: 25–27 January 2009, San Jose, California, United States., 71830X, Proceedings of SPIE, vol. 7183, SPIE, Bellingham, WA, SPIE International Symposium on Biomedical Optics, BIOS 2009, San Jose, California, United States, 24/01/09. https://doi.org/10.1117/12.808792

Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1. / van Rhijn, A.C.W.; Postma, S.; Korterik, Jeroen P. et al.
Multiphoton Microscopy in the Biomedical Sciences IX: 25–27 January 2009, San Jose, California, United States. ed. / Ammasi Periasamy; Peter T.C. So. Bellingham, WA: SPIE, 2009. 71830X (Proceedings of SPIE; Vol. 7183).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

TY - GEN

T1 - Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1

AU - van Rhijn, A.C.W.

AU - Postma, S.

AU - Korterik, Jeroen P.

AU - Herek, Jennifer Lynn

AU - Offerhaus, Herman L.

PY - 2009

Y1 - 2009

N2 - By spectral phase shaping of both the pump and probe pulses in coherent anti-Stokes Raman scattering (CARS) spectroscopy we demonstrate the extraction of the frequencies of vibrational lines using an unamplified oscillator. Furthermore we demonstrate chemically selective broadband CARS microscopy on a mixed sample of 4 μm diameter polystyrene (PS) and poly(methyl methacrylate) (PMMA) beads. The CARS signal from either the PS or the PMMA beads is shown to be enhanced or suppressed, depending on the phase profile applied to the broadband spectrum. Using a combination of negative and positive (sloped) π-phase steps in the pump and probe spectrum the purely non-resonant background signal is removed

AB - By spectral phase shaping of both the pump and probe pulses in coherent anti-Stokes Raman scattering (CARS) spectroscopy we demonstrate the extraction of the frequencies of vibrational lines using an unamplified oscillator. Furthermore we demonstrate chemically selective broadband CARS microscopy on a mixed sample of 4 μm diameter polystyrene (PS) and poly(methyl methacrylate) (PMMA) beads. The CARS signal from either the PS or the PMMA beads is shown to be enhanced or suppressed, depending on the phase profile applied to the broadband spectrum. Using a combination of negative and positive (sloped) π-phase steps in the pump and probe spectrum the purely non-resonant background signal is removed

KW - METIS-259553

KW - Non-linear microscopy

KW - Ultrafast spectroscopy

KW - Coherent anti-Stokes Raman scattering

KW - IR-77975

U2 - 10.1117/12.808792

DO - 10.1117/12.808792

M3 - Conference contribution

SN - 9780819474292

T3 - Proceedings of SPIE

BT - Multiphoton Microscopy in the Biomedical Sciences IX

A2 - Periasamy, Ammasi

A2 - So, Peter T.C.

PB - SPIE

CY - Bellingham, WA

T2 - SPIE International Symposium on Biomedical Optics, BIOS 2009

Y2 - 24 January 2009 through 29 January 2009

ER -

Spectral phase shaping for high resolution CARS spectroscopy around 3000 cm-1

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